Tommy Lee Jones appeared in 1995's Batman Forever as the iconic Batman villain Two-Face AKA Harvey Dent. He performed alongside Jim Carrey's Riddler to double-team Val Kilmer's Batman. In what was a pretty poor movie, Jones' bright and bold Two-Face was one of the better aspects. He's also appeared in two Marvel franchises since then. He's played one of the titular characters, Kevin Brown AKA Agent K, in three Men in Black movies between 1997 and 2012 (Men in Black was published by Marvel in comic book form, believe it or not) and he played the titular character's commanding officer, Colonel Chester Phillips, in Captain America: The First Avenger.